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Tailoring aggregation-induced emission in luminescent solar concentrators through controlled polymerization
2025 / Communications ChemistryLuminescent solar concentrators (LSCs) hold great potential as versatile energy conversion systems for diverse applications. Here, we explore the covalent incorporation of aggregation-induced emission (AIE) luminogens into polymeric backbones for LSCs. Copolymers based on methyl-methacrylate and an AIE-active monomer (tetraphenyl ethylene methacrylate - TPEMA) are ...
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Chiral recognition via symmetry-dependent luminescence in zero-dimensional hybrid copper halides
2025 / Nature CommunicationsChiral recognition through fluorescence changes enables the rapid and sensitive determination of enantiomers. However, the rational design and synthesis of fluorescent probes for efficient chiral recognition remain a challenge. Here we present a novel platform for chiral recognition based on zero-dimensional hybrid copper halides with unique symmetry-dependent pr...
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Polyferrocene-Based Cubosomes: Conversion to Magnetic Mesoporous Microparticles, Supramolecular Modification, and Oxidation Response
2025 / Advanced Functional MaterialsPolymer cubosomes(PCs)areanemergingclassofmesoporousmicroparticles that are produced through solution self-assembly of highly asymmetric block copolymers (BCPs). They proved useful for encapsulation or templating replicas for catalysis and energy storage. Although PCs made from BCPs with intrinsic functions such as response to stimuli, degradation, or coordination ...
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Dual-Mode Thermal Indicator for Cold-Chain Logistics Using Multipiezo Li0.12Na0.88NbO3:Pr3+
2025 / Advanced Optical MaterialsEffective cold-chain monitoring is crucial for safeguarding vaccine quality and efficacy, particularly under harsh sub-zero conditions. However, conventional temperature monitoring frequently encounters challenges, including limited operational performance at low temperatures, narrow tracking windows, susceptibility to photobleaching, and poor reproducibility, seve...
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2Dmaterials, infrared optical synapse, interlayer coupling, orientation de tection, van der Waals heterostructure
2025 / Advanced Photonics ResearchThe all-inorganic lead halide perovskites, including cesium lead iodide (CsPbI3), have attracted significant attention due to their possible applications in photo voltaics, light-emitting devices, and other optoelectronic technologies, driven by their intrinsic optoelectronic properties. This study introduces a simple, green, and scalable solution synthesis method ...
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A Van Der Waals Broadband Infrared Optical Synapse Enabling Orientation Detection
2025 / Advanced ScienceA vision system with efficient infrared-sensitive optical synapses is crucial for enabling infrared radiation detection and target recognition for some predators hunting in the dark. Current 2D synaptic devices typically adopt the strategy of charge trap and release to achieve intelligent sensing and visual recognition. However, the response wavelength is limited i...
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Universal and Nondestructive Direct Photolithography of Colloidal Quantum Dots Using Photocrosslinkable Polymer Blends
2025 / Advanced Functional MaterialsThere has been considerable progress in colloidal quantum dot light-emitting diodes (QD-LEDs) for display applications. However, their commercialization remains challenging, because of the difficulty in achieving high-resolution, full-color patterning of quantum dots (QDs) without degrading their optical properties. Direct photolithography has attracted attention, ...
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Spontaneous dissociation of excitons in polymeric photocatalysts for overall water splitting
2025 / Nature CommunicationsPoly (Triazine Imide) (PTI), like other polymeric semiconductors, suffers from the high exciton binding energy, which intrinsically impedes the separation of photo-induced charge carriers. Herein, we present a crystal structure engineering strategy that exploits the lattice mismatch between the CaCl2 (12) growth template and basal planes of PTI to synthesize unusua...
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Facet-Controlled Growth of Molybdenum Phosphide Single Crystals for Efficient Hydrogen Peroxide Synthesis
2025 / Advanced MaterialsTransition metal phosphides (TMPs) stand out for their excellent catalytic activity, driven by metal‒phosphorus bonding that promotes electron donation, which makes them ideal for electrocatalysis applications. However, the synthesis of single-crystal TMP, which is essential for elucidating intrinsic properties, remains challenging owing to the lack of efficient me...
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Design of circularly polarized phosphorescence materials guided by transfer learning
2025 / Nature CommunicationsIt is highly desirable that artificial circularly polarized phosphorescent materials with high luminescence asymmetry factor (glum), narrowband emission and tunable chiral phosphorescent performance can be constructed. Especially, precise control and simultaneous independent switching of circularly polarized fluorescent and phosphorescent performance for the same...
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A Supramolecular Material for Controlling Kiwifruit Bacterial Canker
2025 / Advanced ScienceKiwifruit, a nutritious fruit consumed globally, is affected by kiwifruit bacterial canker (KBC) caused by Pseudomonas syringae pv. actinidiae (Psa), which is a major biotic stress that adversely impacts its cultivation and production. KBC control is still challenging owing to the evolution of resistant populations of Psa, the environmental risks associated with co...
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The Platform to Characterizing the Thermoelectric Materials by Photo-Crosslinked Ionic Gel Electrolyte
2025 / Advanced Electronic MaterialsAdvances in semiconductor processing have enabled the miniaturization and reduction of power consumption of devices, positioning organic thermoelectric devices—which generate electricity from any heat source—as a promising solution for self-powered microelectronics. To make off-grid electronics more practical, innovative thermoelectric materials with hi...
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Temperature dependency of energy shift of excitonic states in a donor–acceptor type TADF molecule
2025 / Nature CommunicationsIn recent years, thermally activated delayed fluorescence (TADF) has attracted intense attention owing to its straightforward application to high-efficiency organic light-emitting diodes. Further, to develop high-performance TADF materials, many researchers have designed novel molecules that have a small energy gap between the lowest excited singlet and triple...
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Cation-self-shielding strategy promises high-voltage all-Prussian-blue-based aqueous K-ion batteries
2025 / Nature CommunicationsPrussian blue analogues (PBAs) are promising electrode candidates for aqueous batteries because the inevitable interstitial water is generally thought to have little impact on battery performance. Currently, mounting researches have focused on optimizing PBA properties by varying transition metal composition, but less attention has been paid to interstitial water...
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Exceptional Thermal Conductivity in Printed Dielectrics through Compositional and Microstructural Design
2025 / Advanced MaterialsAs electronic devices become simultaneously more powerful and compact, thermal management is increasingly critical. Optimizing components like heatsinks is increasingly required, which has recently leveraged additive manufacturing. There is growing demand to move away from incumbent metallic materials for dielectric materials that are electrically insulative and tr...
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